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Total Synthesis of Brevetoxin A: Part 3: Construction of GHIJ and BCDE Ring Systems

✍ Scribed by K. C. Nicolaou; Guo-qiang Shi; Janet L. Gunzner; Peter Gärtner; Paul A. Wallace; Michael A. Ouellette; Shuhao Shi; Mark E. Bunnage; Konstantinos A. Agrios; Chris A. Veale; Chan-Kou Hwang; John Hutchinson; C. V. C. Prasad; William W. Ogilvie; Zhen Yang

Publisher: John Wiley and Sons
Year: 1999
Tongue: English
Weight: 407 KB
Volume: 5
Category: Article
ISSN: 0947-6539
DOI: 10.1002/(sici)1521-3765(19990201)5:2<628::aid-chem628>3.0.co;2-e

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ChemInform Abstract: Total Synthesis of

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Total Synthesis of Brevetoxin A: Part 1:

Total Synthesis of Brevetoxin A: Part 1: First Generation Strategy and Construction of BCD Ring System

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Total Synthesis of Brevetoxin A: Part 2:

Total Synthesis of Brevetoxin A: Part 2: Second Generation Strategy and Construction of EFGH Model System

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Our second generation strategy for the total synthesis of brevetoxin A involved dissection of the molecule at the ring F oxocene. Synthetically, the F ring formation was expected to occur through Wittig coupling of requisite polycyclic fragments 2 and 3, followed by a hydroxy dithioketal cyclization

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Total Synthesis of Brevetoxin A: Part 4:

Total Synthesis of Brevetoxin A: Part 4: Final Stages and Completion

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