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Photochemistry of titanacyclobutanes. Evidence for a metal-centered 1,4-biradical intermediate

✍ Scribed by Tumas, William; Wheeler, David R.; Grubbs, Robert H.

Book ID: 127320803
Publisher: American Chemical Society
Year: 1987
Tongue: English
Weight: 383 KB
Volume: 109
Category: Article
ISSN: 0002-7863
DOI: 10.1021/ja00254a048

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The formation of products (IV)/(V) and (VIII)/(IX) in the title reactions is explained by either disproportionation or ring closure of an intermediate biradical derived from initial bond formation between the oxygen atom of the aldehyde and the doubly bonded silicon atom of the dimetallene. -(DIXON,