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ChemInform Abstract: Total Synthesis of (+)-Dibromophakellin.

✍ Scribed by Takuya Imaoka; Osamu Iwamoto; Kei-ichi Noguchi; Kazuo Nagasawa

Book ID: 102039162
Publisher: John Wiley and Sons
Year: 2009
Weight: 16 KB
Volume: 40
Category: Article
ISSN: 0931-7597
DOI: 10.1002/chin.200938193

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Total Synthesis of (+)-Dibromophakellin

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Total Synthesis of (+)-Dibromophakellin

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## Abstract **Two members of a family** of pyrrole–imidazole marine alkaloids, (+)‐dibromophakellin and the nonnatural congener (+)‐phakellin, were synthesized enantioselectively from 4‐hydroxy‐L‐proline. The chiral aminal at C10 was constructed efficiently by means of an Overman‐type [3,3] sigmatr

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