Third-order nonlinear optical properties of thin sputtered gold films
β Scribed by E. Xenogiannopoulou; P. Aloukos; S. Couris; E. Kaminska; A. Piotrowska; E. Dynowska
- Publisher
- Elsevier Science
- Year
- 2007
- Tongue
- English
- Weight
- 678 KB
- Volume
- 275
- Category
- Article
- ISSN
- 0030-4018
No coin nor oath required. For personal study only.
β¦ Synopsis
Au films of thickness ranging between 5 and 52 nm were prepared by sputtering on quartz substrates and their third-order nonlinear optical response was investigated by Optical Kerr effect (OKE) and Z-scan techniques using 532 nm, 35 ps laser pulses. All prepared films were characterized by XRD, AFM and UV-VIS-NIR spectrophotometry while their third-order susceptibility v (3) was measured and found to be of the order of 10 Γ9 esu. The real and imaginary parts of the third-order susceptibility were found in very good agreement with experimental results and theoretical predictions reported by Smith et al.
π SIMILAR VOLUMES
Results of wave-dispersed third harmonic generation measurements in sublimed Cso thin films are reported and discussed within a three-level model. Two strong resonant enhancements in cubic susceptibility xc3) ( -3~; o, w, w) are observed. The first one, occurring at a fundamental wavelength of 1.3 p
Third-order nonlinear optical susceptibility, k3) of symmetrically octa-substituted metalfree phthalocyanine thin films measured by the third-harmonic generation technique are reported. The metal-free hthalocyanine has been found to show a 3) ( -3w; 44 m) value as large as 7 . 7 3 ~ lo-'\* esu at 1.
## Abstract __An ultrathin composite film containing anionic AgβHis complexes (His: LβHistidine) and oppositely charged BHβPPV was fabricated by means of the electrostatic layerβbyβlayer selfβassembly technique. UV/Vis spectra showed a continuous deposition process of AgβHis complexes and BHβPPV. T