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Kinetics and the Mechanism of Iron(II) Reduction ofcis-α-halogeno(cetylamine) (triethylenetetramine)cobalt(III) Complex Ion in Aqueous Acid Medium

✍ Scribed by Kannappan Santhakumar; Narayanasamy Kumaraguru; Sankarlingam Arunachalam; Mahadevimanglam Narayanasamy Arumugham

Publisher
Springer
Year
2006
Tongue
English
Weight
328 KB
Volume
31
Category
Article
ISSN
0340-4285

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## Abstract Kinetics of reduction of the surfactant complex ions, __cis__‐chloro/bromo (dodecylamine)bis(ethylenediamine)cobalt(III) by iron(II) in aqueous solution was studied at 303, 308, and 313 K by spectrophotometry method under pseudo‐first‐order conditions, using an excess of the reductant.

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The electron transfer step of the reduction of Mn(acac)s and Co(acac)s by Fe(I1) in acetonitrile is preceded by the one-ended dissociation of an acac ligand and the formation of a binuclear bridged complex. After the electron transfer has taken place through the bridging ligand, the complex dissocia