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ChemInform Abstract: First Highly Regio- and Diastereoselective [3 + 2] Cycloaddition of Chiral Nonracemic Fischer Carbene Complexes with Azomethine Ylides: An Enantioselective Synthesis of (+)-Rolipram.

✍ Scribed by Jose Barluenga; Manuel A. Fernandez-Rodriguez; Enrique Aguilar; Felix Fernandez-Mari; Alejandro Salinas; Bernardo Olano

Publisher: John Wiley and Sons
Year: 2010
Weight: 38 KB
Volume: 33
Category: Article
ISSN: 0931-7597
DOI: 10.1002/chin.200212037

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A new procedure for the synthesis of 1,3,4-trisubstituted and 1,4-disubstituted pyrrolidin-2-one derivatives in an enantioselective fashion is reported. The 1,3-dipolar cycloaddition of (AE)menthol and (À)-8-phenylmenthol derived Fischer alkoxy alkenyl carbene complexes with in situ generated functi

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ChemInform Abstract: First Diastereoselective (3 + 2) Cycloaddition of Chiral Non-Racemic Alkenyl Fischer Carbene Complexes with Diazomethane Derivatives.

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