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The gaseous oxidation of ParaXylene

✍ Scribed by J.A. Barnard; P. Hawtin

Publisher
Elsevier Science
Year
1961
Tongue
English
Weight
483 KB
Volume
5
Category
Article
ISSN
0010-2180

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✦ Synopsis

The gaseous oxidation of para~ylene has been investi~dated in a static ~gstem at temperaturee betwee~t 460 Β° and 512Β°C. The reaction has been followed by pressure change and by chemical analysis of the rex~ctants and products. The reaction ks autocatalytic and it has been shown that formaldeh!tde ~s the degenerate branching intermediate. The order of the reaction varies somewhat u~th mixture compo,~i. tion, but for a fuel/oxygen ratio of 1[2.5, the order with respect to ox?tgen is about 2.0 and with respect to par~ylene edoout 1. O. A mechanism is suggested, based upon the ~enerally accepted scheme for the oxidation o.f methane, which accounts satisfactoril~ for the principal kinetic featuretΒ’ of the reaction.

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