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The effect of a resonance on vibrational structure in the photoelectron spectrum of acetylene

✍ Scribed by R. Unwin; I. Khan; N.V. Richardson; A.M. Bradshaw; L.S. Cederbaum; W. Domcke

Publisher
Elsevier Science
Year
1981
Tongue
English
Weight
334 KB
Volume
77
Category
Article
ISSN
0009-2614

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✦ Synopsis

A nummum m the partial photolonmtlon cross sectlon for the 'nu state of CzHl at hv = 14 eV 1s accompanied by a @cant departure of the viirabonal mtenslties from the Franck-Condon dlstriiutron Usmg an exphclt formula for resonant photoermssion we show with mode! calcuht~ons that a resonance ==3 eV above the first lonisatlon potential IS responsible for this effect.

πŸ“œ SIMILAR VOLUMES

Multiple excitations in the core photoel
Multiple excitations in the core photoelectron spectrum of acetylene
✍ Reidar Arneberg; Hans Γ…gren; Per-Γ…ke Malmquist; Svante Svensson πŸ“‚ Article πŸ“… 1982 πŸ› Elsevier Science 🌐 English βš– 412 KB

A h&h-resolution core photoelecrron spectrum of free ncetylcne is presented. Con@unbon mk?ractlon and complete acme space SCF calculanons were carned out for awgnment and predIctIon of encrges and tntcns~ues UI the spectrum The shake-up structure 15 found to be strongly dommatcd by rntervaknce I,, 1