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The 99Ru Mössbauer spectrum of β-RuCl3

✍ Scribed by F.M. Dacosta; T.C. Gibb; R. Greatrex; N.N. Greenwood

Publisher
Elsevier Science
Year
1975
Tongue
English
Weight
230 KB
Volume
36
Category
Article
ISSN
0009-2614

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✦ Synopsis

The 99Ru nuclear quadrupole interaction in pRuC13 can be related to the large irigonal distortion at the ruthenium site.

The ratio of the quadrupole moments has been determined to be Qe/Qg = +3.06 + 0.10, and it is confirmed that Qe and Qg arc both positive.

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The MGssbauer spectrum of the [Fe(NR3)6]'+ cation consists of a single narrow line at room temperature \_ This musud effect is attributed to the existence of a dynamic Jahn-Teller distortion which inverts the t2g orb%& very rapidly such that the time-averaged qvdence is zero. The observed splitting