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Synthesis of isoquinuclidinones via a tandem amination/imination sequence: application to the synthesis of (−)-mearsine

✍ Scribed by James D. Cuthbertson; Andrew A. Godfrey; Richard J.K. Taylor

No coin nor oath required. For personal study only.

✦ Synopsis

in recognition of his many seminal achievements in organic chemistry and his friendship over numerous years of Tetrahedron Board Meetings.

📜 SIMILAR VOLUMES

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## Abstract The sequence converts 6‐acyl‐cyclohex‐2‐enones of type (I) directly to the required isoquinuclidinones.

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The addition of allylcopper reagents to imines derived from S-valine occurs with excellent diastereoselectivity (e.e. 98 %).

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