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Structures of some moenomycin antibiotics - inhibitors of peptidoglycan biosynthesis

✍ Scribed by Jürgen Scherkenbeck; Aranka Hiltmann; Kurt Hobert; Wassja Bankova; Torsten Siegels; Manfred Kaiser; Dietrich Müller; Hans Jürgen Veith; Hans-Wolfram Fehlhaber; Gerhard Seiberg; Astrid Markus; Michael Limbert; Gerhard Huber; Dirk Böttger; Andreas Stärk; Shuji Takahashi; Yveline van Heijenoort; Jean van Heijenoort; Peter Welzel

Publisher
Elsevier Science
Year
1993
Tongue
French
Weight
742 KB
Volume
49
Category
Article
ISSN
0040-4020

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✦ Synopsis

w -Isolation, structural assignment, and anhblotlc efficiency of the new moenomycm antiblohcs C3 (lb) and C4 (lc) IS decnbcd The previously pubhshcd structure of phohpomycm (ld) 1s modified Zntroduction The fanuly of moenomycm-type antibiotics includes the components of the flavomycmR complex, the prasmomycms, diumycms (marcarbomycms), 11837 R P , 8036 R.P (quebemecm), 19402 R P ,

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The C 25 terpenoid moenocinol is suggested to originate from a farnesyl precursor and geranyl pyrophosphate. The new mechanism is in accord with all previous feeding experiments. Feeding of [2,[5][6][7][8][9][10][11][12][13] C 2 ]-labeled 1-deoxy-D-xylulose proves how the two units are joined in the