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Sequential Copper-Catalyzed Rearrangement–Allylic Substitution of Bicyclic Hydrazines with Grignard Reagents

✍ Scribed by Stefano Crotti; Ferruccio Bertolini; Franco Macchia; Mauro Pineschi

Publisher
John Wiley and Sons
Year
2009
Tongue
English
Weight
181 KB
Volume
351
Category
Article
ISSN
1615-4150

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## Abstract The __ortho__‐diphenylphosphanylbenzoyl (__o__‐DPPB) group was explored as a directing leaving group in copper‐mediated and copper‐catalyzed allylic substitution with Grignard reagents. Complete control of chemo‐, regio‐ and stereoselectivity with complete __syn__‐1,3‐chirality transfer