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Resonance CARS in Br2

✍ Scribed by Ilse Aben; Wim Ubachs; Gert van der Zwan; Wim Hogervorst

Publisher
Elsevier Science
Year
1992
Tongue
English
Weight
578 KB
Volume
198
Category
Article
ISSN
0009-2614

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✦ Synopsis

Intense CARS spectra were observed in bromine vapour, which could be attributed to resonances in the molecular as well as atomic species. From accurate measurements of frequency positions and polarization dependencies a vibrational overtone sequence Av= 2-12, characteristic for resonance CARS, was identified for Br2. Doublets of rotational lines reveal enhancement by discrete transitions between bound states in the molecular medium.

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