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Femtosecond time-resolved resonance CARS theory

✍ Scribed by Valey F. Kamalov; Yuri P. Svirko

Publisher
Elsevier Science
Year
1992
Tongue
English
Weight
580 KB
Volume
194
Category
Article
ISSN
0009-2614

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✦ Synopsis

A femtosecond time-dependent resonance CARS theory is developed. The resonance CARS response is calculated in the temporal representation on the basis of density-matrix equations. Two experimental schemes for the study of relaxational processes in excited electronic states which use time-delayed femtosecond pulses are discussed. The simple mode1 of wavepacket temporal evolution is used for the calculation of the CARS depolarization ratio.

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