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Rate coefficients at 297 K for proton transfer reactions with H2O. Comparisons with classical theories and exothermicity

✍ Scribed by D. Betowski; J.D. Payzant; G.I. Mackay; D.K. Bohme

Publisher: Elsevier Science
Year: 1975
Tongue: English
Weight: 447 KB
Volume: 31
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(75)85030-5

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Rate constants for proton transfer reactions of the type XH+ + NH3 -NH: + X where X = Hz. NH2. CH4, HzO, CO, N2, CzH4, CzH6, C3H.5, NzO and CaHs have been measured at 297°K using the flowing afterglow technique. These rate constants and others measured previously in this laboratory for proton transf

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Rcccivcd 30 Apnl 1982 SO:, photodissociation at 193 nm (AIF cxclmer lmr) ha been used to create SO radicals; the chcmdumincsccncc from the SO + 03 reaction has been used to follow the SO ndical decay. Rate coefticicnls at 298 K of (1 07 t 0.16) x 10-r6, (1 06 f 0 16) x 10-r3, and (1 48 k 0 20) x IO-

Rate coefficients for CS reactions with

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CS radicals have been produced by photodissociation of CS2 at 193 MI and their disappearance monitored by LIF\_ The vibrationally excited CS radicals rapidly relax to CS(v = 0). At 298 K, the rate coeffkients for CS(u = 0) reactions with 02, 03 and NO\* are (2.9 +\_ 0.4) x lo-", (3.0 + 0.4) X lo-I6

Rate coefficients and product ion distri

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The rdt, cocii~c~cnts and product eon dlsrrlbutlons for rhc reactions ot OH\* and tlzO+ u ith N2\_ 02 h'0 X20 Xc, CO, CO? H2S Jnd 112 hd\c been dctermlned it 194 + 2 K usmg a selcctcd ton ilo\. rubc (SIFT) dppclrnrus These reactIons urre generally found to proLccd b\~ athcr proton or charge trsnsfcr

Rate constants at 295 K for the reaction

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Constants of the rawions of Cl with HIOz. IX&, 03, CH4, and HNC)J wertt mezxured at 295 K using a flaw discharge-mass spectrometric method. The rate consmts are, WpectiveIy, (6.2 ?c I.51 X 10qzS, (32&) x 10"tl, (1.3 -+. 0.3) X lo-'t, (1.2 ?t 0.3) X 10-13, and (6.8 t 3.4) X lO-is cm3/s.