✦ LIBER ✦

Photoelectrons from negative dimers and clusters of sulfur dioxide

✍ Scribed by T. Dresch; H. Kramer; Y. Thurner; R. Weber

Publisher: Elsevier Science
Year: 1991
Tongue: English
Weight: 481 KB
Volume: 177
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(91)85070-d

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✦ Synopsis

Photoelectrons originating from sulfur dioxide cluster anions were studied using a tandem mass spectrometer combined with an electron detector and intracavity argon-ion and dye lasers. The absolute photodetachment cross section of the dimer anion increases to (8 k 1) x 1 O-I9 cm2 at 2.7 I eV photon energy. Electrons detected from the interaction of photons with sulfur dioxide clusters wcrc found to be produced in sequential two-step processes only, revealing a lower bound of the cluster's detachment threshold energy of 2.7 eV.

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