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Photodissociation Dynamics of SOCl2.

โœ Scribed by Alexei Chichinin; Tina S. Einfeld; Karl-Heinz Gericke; Joerg Grunenberg; Christof Maul; Lars V. Schaefer

Publisher
John Wiley and Sons
Year
2005
Weight
9 KB
Volume
36
Category
Article
ISSN
0931-7597

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Dynamics of photodissociation
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Using a sudden transition state theory we find that photodissociation of long-lived resonances of DzH+ leads to the H+ fragment for total angular momentum JC 27 while D+ is formed for J> 30. This quantum result which is critically dependent on the difference of zero-point energies between D2 and HD

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Photodissociation of HrS in krypton matrices is followed by monitoring laser-induced fluorescence from the SH photofragment. No evidence of an energy threshold for dissociation is observed. Quantum yields of dissociation, referenced to gas-phase absorption cross sections, increase nearly linearly fr