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Overlapping resonances in the control of intramolecular vibrational redistribution

✍ Scribed by Gerbasi, D.; Sanz, A. S.; Christopher, P. S.; Shapiro, M.; Brumer, P.

Book ID
121275746
Publisher
American Institute of Physics
Year
2007
Tongue
English
Weight
465 KB
Volume
126
Category
Article
ISSN
0021-9606

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πŸ“œ SIMILAR VOLUMES

On the selective elimination of intramol
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A method is proposed Tor the sclafive elimination of in~ramolccular wbralional redwribunon (IVR) in polyalomic molecules by using a strong resonant laser excitation. When the Rabi frequency is larger than the Irquenq spread of an isolated group of molecular eigenstale IVR prw se totally suppressed.

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The fluorescence decly of pyrene vapour, excited into the SI-state with a frequency doubled ruby-&r pulse : (28800 an-') .has been studio unda conditions where the excited molearles are c4lisionally unperturbed. The fluorescence decay curye can be de&i as a Sum of two exponential components. The ch&