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Nickel-Catalyzed Enantio- and Diastereoselective Three-Component Coupling of 1,3-Dienes, Aldehydes, and a Silylborane Leading to α-Chiral Allylsilanes

✍ Scribed by Dr. Nozomi Saito; Ayami Kobayashi; Prof. Dr. Yoshihiro Sato

Book ID: 111999474
Publisher: John Wiley and Sons
Year: 2011
Tongue: English
Weight: 371 KB
Volume: 124
Category: Article
ISSN: 0044-8249
DOI: 10.1002/ange.201107360

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A nickel-catalyzed diastereoselective alkylative three-component coupling of 1,3-diene and aldehyde with organoboron or organosilicon reagents has been realized. The diastereoselectivity was dramatically changed depending on the class of organometallic reagents. The reaction using ArB(OH) 2 in the p