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Master Equation Models for the Pressure- and Temperature-Dependent Reactions HO + NO 2 → HONO 2 and HO + NO 2 → HOONO

✍ Scribed by Golden, David M.; Barker, John R.; Lohr, Lawrence L.

Book ID
121229105
Publisher
American Chemical Society
Year
2003
Tongue
English
Weight
312 KB
Volume
107
Category
Article
ISSN
1089-5639

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## Abstract A theoretical analysis of the temperature and pressure dependence of the reaction HO + NO~2~ + M ⇔︁ HONO~2~ + M is made over the temperature range 50–1400 K and the pressure range 10^−4^–10^3^ bar where experimental data are available. The treatment accounts for contributions from anhar

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Mixtures of N20, Hz, 0 2 , and trace amounts of NO and NO2 were photolyzed at 213.9 nm, at 245'-328'K, and at about 1 atm total pressure (mostly H2). HO2 radicals are produced from the photolysis and they react as follows: (la) Reaction (lb) is unimportant under all of our reaction conditions. Rea