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Mass-resolved VUV laser spectra in the vicinity of the Rydberg minimum of the 1 1∑+u state of Cl2

✍ Scribed by P. Wang; I.V. Okuda; S.S. Dimov; R.H. Lipson

Publisher
Elsevier Science
Year
1994
Tongue
English
Weight
592 KB
Volume
229
Category
Article
ISSN
0009-2614

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✦ Synopsis

Excitation spectra of the 1 'x:,' tX 'xc transition of Cl2 near 136 nm are presented. Jet-cooled molecules were excited with a tunable vacuum ultraviolet laser generated by four-wave difference-mixing in Kr, and the resultant photoions were mass discriminated in a time-of-flight spectrometer. Rotationally resolved transitions for vibrational levels localized in the Rydberg Portion of the l-state double well potential were recorded and analyzed for all three naturally occurring Cl2 isotopomers.

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