The lifetimes of rotationally cooled NO, were measured in the spectral region 5710-5960 A in a differentially pumped collision-free supersonic molecular beam. Lifetime values (rotationally independent) between 75 and 260 ps were obtained. Over narrow spectral regions, the product of the fluorescenc
Long radiative lifetimes of SO2 in a collision-free supersonic molecular beam
✍ Scribed by Ofer Snè; Ori Cheshnovsky
- Publisher
- Elsevier Science
- Year
- 1986
- Tongue
- English
- Weight
- 559 KB
- Volume
- 130
- Category
- Article
- ISSN
- 0009-2614
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✦ Synopsis
Radiative lifetimes and delayed laser-induced fluorescence spectra of cold SO2 were measured in the range 3000-3150 A in a differentially pumped collision-free supersonic beam. Lifetimes between 9 and 300 ps were obtained. We show the existence of high-density, low-intensity, and long-lifetime states in the vicinity of the strong spectral transitions.
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