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Ion/molecule reactions with S2F10: detection of S2F·+10, S2F+11 and two isomers of SF+5

✍ Scribed by Gholamreza Javahery; Hansjürgen Becker; Michail V. Korobov; Milton Farber; David Cooper; Diethard K. Bohme

Book ID: 107920625
Publisher: Elsevier Science
Year: 1994
Tongue: English
Weight: 751 KB
Volume: 133
Category: Article
ISSN: 0168-1176
DOI: 10.1016/0168-1176(94)03951-8

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Data on the kinetics of S,F,, pyrolysis, which gives SF, + SF, , have been reinterpreted to give a value for the equilibrium constant of S,FIo SF, + SF, . This, together with statistical estimates of the entropy and heat capacity of S,F,, , can be used to give for this reaction values of AH,.,, = 19

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The reaction of CzF5 radicals with HzS (2) C2F5 + HzS -+ CzF5H + HS kfi was studied over the range 1"-123"C using CZFS radicals generated by photolysis of perfluoropropionic anhydride. The rate constant k~ for reaction (2) is given by where e = 2.303RT/cal mole-'. The relevance of this result to c