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Highly Enantioselective Palladium-Catalyzed Alkylation of Acyclic Amides

✍ Scribed by Kai Zhang; Qian Peng; Xue-Long Hou; Yun-Dong Wu

Publisher: John Wiley and Sons
Year: 2008
Tongue: English
Weight: 332 KB
Volume: 120
Category: Article
ISSN: 0044-8249
DOI: 10.1002/ange.200704629

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## Abstract Lithium and magnesium enolates of cyclohexanone undergo palladium‐catalyzed allylic alkylations under mild conditions. Diastereoselectivity and enantioselectivity are observed when the diphenyl‐ and dimethyl‐substituted allylic substrates **1a** and **1b** are reacted with cyclohexanone