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Experimental and Theoretical Studies of the Reaction of the OH Radical with Alkyl Sulfides: 3. Kinetics and Mechanism of the OH Initiated Oxidation of Dimethyl, Dipropyl, and Dibutyl Sulfides: Reactivity Trends in the Alkyl Sulfides and Development of a Predictive Expression for the Reaction of OH with DMS

✍ Scribed by Williams, M. B.; Campuzano-Jost, P.; Hynes, A. J.; Pounds, A. J.

Book ID
127022693
Publisher
American Chemical Society
Year
2009
Tongue
English
Weight
954 KB
Volume
113
Category
Article
ISSN
1089-5639

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✍ I. Barnes; V. Bastian; K. H. Becker πŸ“‚ Article πŸ“… 1988 πŸ› John Wiley and Sons 🌐 English βš– 936 KB

The rate constant of the reaction of OH with DMS has been measured relative to OH + ethene in a 420 1 reaction chamber a t 760 torr total pressure and 298 t 3 K in N L + 0, buffer gas using the 254 nm photolysis of H202 as the OH source. In agreement with a recent absolute rate determination of the

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The gas phase reaction of OH radicals with dimethyl sulfide (CH,SCH,, DMS) has been studied using both an absolute and a relative technique a t 295 2 2 K and a total pressure of 1 atm. The absolute rate technique of pulse radiolysis combined with kinetic spectroscopy was applied. Using this techniqu