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Dual mechanism of zinc-proline catalyzed aldol reactions in water

✍ Scribed by Kofoed, Jacob; Darbre, Tamis; Reymond, Jean-Louis

Book ID
121426418
Publisher
Royal Society of Chemistry
Year
2006
Tongue
English
Weight
122 KB
Volume
14
Category
Article
ISSN
1359-7345

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Computational Evidence for the Enamine M
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Theoretical evidence now suggests that the mechanism of the longdebated Hajos-Parrish-Eder-Sauer-Wiechert reaction, the prototype for asymmetric organocatalytic reactions, involves a proline enamine intermediate (center) which undergoes a concerted aldol cyclization with proton transfer. For more de