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Direct Catalytic Asymmetric Vinylogous Mannich-Type Reaction of γ-Butenolides with Ketimines

✍ Scribed by Yin, Liang; Takada, Hisashi; Kumagai, Naoya; Shibasaki, Masakatsu

Book ID: 120541402
Publisher: John Wiley and Sons
Year: 2013
Tongue: English
Weight: 447 KB
Volume: 52
Category: Article
ISSN: 0044-8249
DOI: 10.1002/anie.201303119

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## Abstract **Weich hilft hart**: Die Titelreaktion zwischen Thioamiden und __N__‐(Diphenylphosphinoyl)iminen nutzt die kooperative Katalyse einer weichen Lewis‐Säure und einer harten Brønsted‐Base, um Thioamid‐Kohlenstoff‐Pränucleophile in Mannich‐Produkte zu überführen (siehe Schema). Folgereakti