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Deactivation of O2(1Δg)

✍ Scribed by F.D. Findlay; C.J. Fortin; D.R. Snelling

Publisher
Elsevier Science
Year
1969
Tongue
English
Weight
281 KB
Volume
3
Category
Article
ISSN
0009-2614

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roughly4 x10-19 a room temperature rate constant of 2.2 f 0.5 L: 10-18 cm3 molec-1 se~-~ by 02 and cm3 molec-1 set-1 by dry air. Deactivation by N2 proceeds at least an order of magnihrde more slowly.

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Relaxation rates for 02('&+) by nonradiative pathways have been determined using the fast-flow technique. 02 ('\3,+) is formed from 0 2 ( l A g ! by an energy pooling process. 02('AK) is generated by passing purified oxygen through a microwave discharge. Oxygen atoms are removed by distilling mercur

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In a fast flow system mixtures of SOCI 2 with helium were passed through a microwave discharge and added downstream to a flow of metastable 02 (lAg) molecules. Chemiluminescence of the SO(IAg--aZg) (0,0) band was observed at 1.705 #m in addition to the already known (0,0), (0,1), (1,1), and (2,2) ba

Rate constants of O2(1Δg)
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The rate constants of OY('As) with aliphatic alcohols, terpenes, unsaturated hydrocarbons, chlorinated hydrocarbons, oxygen, and diamines have been studied in the presence of NO,. The rate constants for oxygen, 1.2-ethane diamine, and 1,2-propane diamine are (9.9 ? 0.4) x lo2, (8.7 t 0.7) x lo4, and