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Covalency from quadrupole coupling in ABCI3 systems

โœ Scribed by W.B Euler; L.E Mohrmann Jr.; B.B Garrett

Book ID
103186921
Publisher
Elsevier Science
Year
1979
Weight
517 KB
Volume
35
Category
Article
ISSN
0022-2364

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The quadrupole interaction has been measured by ESR spectroscopy for the paramagnetic centers in irradiated KC103 zmd NaC103 which have previously been associated with ClOa radicals. The observed cylindriul quadrupole coupling is e2qQ = 42 + 3 MHz. a value consistent with the field gradient obtained

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K = 1 + 0 transitions in CHsOD for / = 1, 2, 3 and 4 E,-type states were measured using a beam maser spectrometer with 6 kHz linewidth (fwhm). Analysis of J = 1 and / = 2 spectra provided a deuterium quadrupole coupling strength along the O-D bond di?ection of eqzzQ = 303 i 12 kHz.