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Classical formalism for a translational—rotational energy transfer mechanism in atom—diatom collisions

✍ Scribed by Aristophanes Metropoulos

Book ID
107732932
Publisher
Elsevier Science
Year
1982
Tongue
English
Weight
471 KB
Volume
89
Category
Article
ISSN
0009-2614

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📜 SIMILAR VOLUMES

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Values of average energy transferred, (AC). and average energy loss, (h),, per collision were calculated from classical trajectories for collinear A\*+ M collisions in which A2 is highly vibrationally excited. Results were compared with those from the singleencounter impulsive collision model, from

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Cross sections and rate constants for the inelastic collision, OH(A2Z+,v=I,j=15) + Ar ~ OH(A2 r.+,v=0,]=20) + Ar, have been calculated in the infinite-order sudden (IOS) and distorted-wave (DW) approximations. The results agree well with experiment.

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A study of the vibration-translation energy transfer in atom-diatom collinear collisions is made. Using an algebraic approach developed by Gazdy and Micha, the time evolution operator of the linearly driven parametric oscillator (LDPO) is obtained, and used to transform the cubic part of the interac