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Chiral Diphosphites and Diphosphoramidites as Cheap and Efficient Ligands in Rh-Catalyzed Asymmetric Olefin Hydrogenation.

✍ Scribed by Manfred T. Reetz; Gerlinde Mehler; Oleg Bondarev

Publisher: John Wiley and Sons
Year: 2006
Weight: 31 KB
Volume: 37
Category: Article
ISSN: 0931-7597
DOI: 10.1002/chin.200641059

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Several years ago it was reported that monodentate phosphites, [1] phosphonites, [2] and phosphoramidites [3] derived from 2,2'-dihydroxy-1,1'-binaphthyl (BINOL) are efficient ligands in various Rh-catalyzed asymmetric olefin-hydrogenation reactions (90-99 % ee). These observations were surprising,