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Catalytic Enantioselective Intermolecular Cycloaddition of Diazodiketoester-Derived Carbonyl Ylides with Indoles Using Chiral Dirhodium(II) Carboxylates

✍ Scribed by Shimada, Naoyuki; Oohara, Tadashi; Krishnamurthi, Janagiraman; Nambu, Hisanori; Hashimoto, Shunichi

Book ID
126870755
Publisher
American Chemical Society
Year
2011
Tongue
English
Weight
823 KB
Volume
13
Category
Article
ISSN
1523-7060

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Enantioselective 1,3-dipolar cycloaddition of the ester-carbonyl ylides derived from methyl 2-(diazoacetyl)benzoate and 3-(diazoacetyl)-2-naphthoate with dipolarophiles has been eected with the aid of dirhodium(II) tetrakis[N-phthaloyl-(S)-tert-leucinate], aording cycloadducts in up to 93% ee.

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