The feasibility of determining nuclear quadrupole hyperfine splittings in the ground electronic state of a polyatomic molecule using a double resonance quantum beat method has been demonstrated. Pyrimidine molecules were coherently excited into single rotational states of the So 201 ( 13a ~) vibrati
✦ LIBER ✦
Zeeman quantum beat in nuclear quadrupole resonance probed by Raman heterodyne spectroscopy
✍ Scribed by Xing-Fei He; Peter T.H. Fisk; Neil B. Manson
- Publisher
- Elsevier Science
- Year
- 1992
- Tongue
- English
- Weight
- 241 KB
- Volume
- 53
- Category
- Article
- ISSN
- 0022-2313
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## Abstract The dideprotonation of 4‐(4‐nitrophenylazo)resorcinol generates an anionic species with substantial electronic π delocalization. As compared to the parent neutral species, the anionic first excited electronic transition, characterized as an intramolecular charge transfer (ICT) from the