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Unimolecular chemistry of methyl formate cation radical. A combined theoretical and experimental study

โœ Scribed by Heinrich, Nikolaus; Drewello, Thomas; Burgers, Peter C.; Morrow, J. Charles; Schmidt, Jochen; Kulik, Willem; Terlouw, Johan K.; Schwarz, Helmut

Book ID
126200772
Publisher
American Chemical Society
Year
1992
Tongue
English
Weight
1003 KB
Volume
114
Category
Article
ISSN
0002-7863

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Unimolecular chemistry of oxazole and is
Unimolecular chemistry of oxazole and isoxazole radical cations in the gas phase: Combined experimental and molecular orbital study
โœ R. Flammang; M. Plisnier; G. Bouchoux; Y. Hoppilliard; S. Humbert; C. Wentrup ๐Ÿ“‚ Article ๐Ÿ“… 1992 ๐Ÿ› John Wiley and Sons ๐ŸŒ English โš– 837 KB

Molecular radical cations of oxazole (1) and isoxazole (2) dissociate by losing carbon monoxide or a hydrogen atom, respectively. These fragmentations were examined by use of tandem mass spectrometry, flash vacuum pyro- lysis and ab initiu molecular orbital calculations. A multi-step mechanism is pr