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Two approaches to stochastic rate theory

✍ Scribed by S. G. Christov

Publisher
John Wiley and Sons
Year
1997
Tongue
English
Weight
183 KB
Volume
64
Category
Article
ISSN
0020-7608

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✦ Synopsis

A comparison is made between two approaches to a Kramers-type reaction rate theory. The usual one is based on a linear coupling model between a particle and the medium oscillators. Use is made of two different separable reaction coordinates in the absence and presence of coupling, respectively. A more general model consists of Ε½ . assuming an arbitrary nonlinear coupling between the reactant and medium, making Ε½ . use of a single curvilinear reaction coordinate of the entire many-dimensional system Ε½ . reactant q medium . A comparison with the exact dynamic rate theory is made, showing its equivalence with the generalized stochastic theory.

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