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Towards the total synthesis of colletofragarones: constructing the macrocyclic lactone by high pressure-mediated intramolecular Diels–Alder reaction

✍ Scribed by Joaquín G. Marrero; Laurence M. Harwood

Publisher
Elsevier Science
Year
2009
Tongue
French
Weight
418 KB
Volume
50
Category
Article
ISSN
0040-4039

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✦ Synopsis

We report herein an intramolecular Diels-Alder approach towards the construction of the macrocyclic lactone ring and the perhydrobenzofuran system of the colletofragarones, novel metabolites produced by fungi of the genus Colletotrichum that are responsible for inhibition of germination of the conidia in these species.

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