Theoretical study of the energy spectra of multiphoton above-threshold dissociation of H2+ in intense laser fields
โ Scribed by Dimitry A. Telnov; Shih-I Chu
- Publisher
- Elsevier Science
- Year
- 1996
- Tongue
- English
- Weight
- 596 KB
- Volume
- 255
- Category
- Article
- ISSN
- 0009-2614
No coin nor oath required. For personal study only.
โฆ Synopsis
We present a new procedure for the determination of the kinetic energy spectra of molecules undergoing multiphoton above-threshold dissociation (ATD) in intense laser fields. The method is based on the extension of the non-Hermitian Floquet theory and an integral equation formulation of the partial rates. The non-Hermitian Floquet Hamiltonian is discretized by means of the complex-scaling generalized pseudospectral technique, and a back rotation procedure is introduced for extracting the partial widths from the total resonance wavefunctions. The method is applied to the study of the ATD energy spectra of H~-molecular ions in intense (775 nm) laser fields.
๐ SIMILAR VOLUMES
We present a brief account of some recently developed generalized Floquet methods (both time-dependent and time-independent) for the nonperturbative treatment of the time-development of wavefunctions or the density matrix operator of quantum systems driven by intense periodic or multi-color (multi-f
CH(A \*A-X %) emission was observed following multiple photon dissociation of ketene with an ArF laser. For rotational levels with N' from 14 to 19 the symmetric A component of the emission had higher intensity than the antisymmetric and the opposite was observed for levels with N' between 20 and 23