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The photoelectron spectrum of thiazyl fluoride

✍ Scribed by R.N. Dixon; G. Duxbury; G.R. Fleming; J.M.V. Hugo

Publisher: Elsevier Science
Year: 1972
Tongue: English
Weight: 334 KB
Volume: 14
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(72)87141-0

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✦ Synopsis

The phctoeIectron spectrum has Seen observed using He 584 a excitation.

.rhssignments are made and compared with those for related molecules. . Thiazyl .fluoride, NSF, is isoefectronic with sufphur dioxide SO,. A comparison between the electronic structures of these molecules is of considerable theeretical iriterest since the bonti stretching force constants are well represented by the very different valence-bond formulae NZ&F and O=S=O. Work by Barrow et al. [?,2] on the electronic spectrum of NSF showed that the variations of the geometry on eiectronic excitation from the ground state are at variance with Walsh's rules {3]. It is suspected that in the corresponding SO, transitions [4,p.605],

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