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The effect of pressure on the equilibrium in the Diels–Alder reaction between 9-chloroanthracene and tetracyanoethylene

✍ Scribed by Vladimir D. Kiselev; Elena A. Kashaeva; Alexander I. Konovalov

Book ID
111730105
Publisher
Royal Society of Chemistry
Year
1998
Tongue
English
Weight
125 KB
Volume
8
Category
Article
ISSN
0959-9436

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Pressure effect on the rate and equilibr
Pressure effect on the rate and equilibrium constants of the Diels-Alder reaction 9-chloroanthracene with tetracyanoethylene
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The pressure effect on the forward and backward rate constants and equilibrium constants of the Diels-Alder reaction of 9-chloroanthracene with tetracyanoethylene has been investigated in 1,2-dichloroethane up to 1000 kgcm -2 at 298.15 K. The reaction volume obtained from the pressure effect on equi

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The activation and reaction volumes (∆V /∆V) were showing negative volumes of activation (∆V Ͻ 0) whereas the others are slightly retarded (∆V Ͼ 0). From the analysis determined for the retro Diels-Alder reactions of the parent dihydrobarrelene 1a, its 2-cyano derivative 1b, the exo and of the volum