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The dynamics of the reaction: O(1D2) + H2S → OH(ν′) + HS

✍ Scribed by E.J. Kruus; B.I. Niefer; J.J. Sloan

Book ID
108043364
Publisher
Elsevier Science
Year
1991
Tongue
English
Weight
811 KB
Volume
57
Category
Article
ISSN
1010-6030

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Dynamic aspects of the reaction O(1D) +
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The rate constant for the reaction between OH and vibrationally excited H2, OH + H 2 (v = 1) ~ H20 + H, has been measured directly at 298 K. kol is found to be (7.5 -+ 3) X 10 -13 cma/molecule s, corresponding to a vibrational rate enhancement ofkol/koo = (1.2 -+ 0.4) X 102.

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The product hydroxyl radical arising from the reaction 0( 1D 2)-t-H 2 ---, OH + H was detected by LIF following excitation of the off-diagonal transition OH(A2E +, v' = 1 6-X 2II, v" = 2) in the region 348-357 nm. The rotational population distribution in v" = 2 appears to be inverted and quite simi