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The Chemistry of Thujone. Part XIV.. Synthesis of biologically active aryl terpenoid analogues

✍ Scribed by Chris Carvalho; William R. Cullen; Michael D. Fryzuk; Helen Jacobs; Brian R. James; James P. Kutney; Krystyna Piotrowska; Vinod K. Singh

Publisher
John Wiley and Sons
Year
1989
Tongue
German
Weight
503 KB
Volume
72
Category
Article
ISSN
0018-019X

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## Abstract The thujone derived enone **1** is converted in one step to the pentacyclic compound **4**. The structure of **4** was determined by X‐ray diffraction analysis. The acid‐catalyzed cyclopropane‐ring opening of **4** and of the model compound **9** are described.

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## Abstract The thujone‐derived enone **1**, upon base‐catalyzed reaction with 2‐methyl‐6‐vinylpyridine is converted to the pyridine analogue **5** __(Scheme 1)__. Catalytic reduction of the latter to **6** generates two new centers of chirality which eventually become C(8) and C(14) in the ultimat

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