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Synthesis, structures and electrochemistry studies of 2Fe2S–Fe(ii)(S–2N)2 models for H-cluster of [FeFe]-hydrogenase

✍ Scribed by Hu, Ming-Qiang; Wen, Hui-min; Ma, Cheng-Bing; Li, Na; Yan, Qing-Yun; Chen, Hui; Chen, Chang-Neng

Book ID: 111687598
Publisher: Royal Society of Chemistry
Year: 2010
Tongue: English
Weight: 166 KB
Volume: 39
Category: Article
ISSN: 1477-9226
DOI: 10.1039/c0dt00505c

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## Abstract Electrochemical investigations on a structural analogue of the [2Fe]~H~ subsite of [FeFe]H~2~ases, namely, [Fe~2~(CO)~6~{μ‐SCH~2~N(CH~2~CH~2~‐ OCH~3~)CH~2~S}] (1), were conducted in MeCN/NBu~4~PF~6~ in the presence of HBF~4~/Et~2~O or HOTs. Two different catalytic proton reduction proce