Cryorolling was performed on commercially pure aluminium sheet from an initial thickness of 7 mm to 0.25 mm with a total true strain of around 3.33. Cryorolling was performed in many passes with only 5% reduction in each pass to avoid adiabatic heating during rolling process. Detailed Transmission Electron Microscopic studies showed increased dislocation density and distributed dislocation cell structure. Streaks along with ring pattern in selected area electron diffraction of transmission electron microscopy evidenced the existence of texture component on the surface of rolled sheet along with nanocrystalline sub-structure. Studies on fracture behavior of the cryorolled sheets were performed using specimen of double edge-notch tensile geometry. Compared to the conventionally rolled sheet metal, the strain triaxiality ratio value in the case of cryorolled sheets is insensitive to the void growth analysis due to the presence of nano-sized grains. The ratio of length to the width of voids varies from 1.6 to 2.4 in the case of conventionally rolled sheet. In contrast, length to width ratio is very close to 1.0 in the case of cryorolled sheet. Thus no oblate or prolate voids were observed during cryorolling compared with conventionally rolled sheets and it is observed the formation of equiaxed nanostructured grains. In the case of cryorolled sheets, minimal variation in length to width ratio was observed with the variation in the shear strains, due to the presence of nanostructured grains. Whereas, in the case of conventionally rolled material, wide variation in the length to width ratio with the variations in the shear strains was observed.