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Studies on the oxidation mechanism of H2S based on direct examination of the key reactions

✍ Scribed by Kentaro Tsuchiya; Kenshu Kamiya; Hiroyuki Matsui

Publisher
John Wiley and Sons
Year
1997
Tongue
English
Weight
193 KB
Volume
29
Category
Article
ISSN
0538-8066

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✦ Synopsis

numbers of studies were performed until very recently on the fundamental oxidation reaction mechanism of hydrogen sulfide and related H 9 S 9 O reaction systems.

The oxidation process of H 2 S (and some times the catalytic effect of SO 2 ) have been investigated in several flame studies [1 -5], and the reaction mechanisms were discussed based on the measured product distributions. These studies have provided much useful information on the elementary reactions of H 9 S 9 O systems, however, it is generally very difficult to judge the reliability of kinetic/thermodynamic parameters of individual elementary reactions proposed in these indirect studies. It is also noted that even a conventional shock tube study was not performed for clarifying oxidation mechanism of H 2 S (as far as we know), except an ignition delay mea-

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