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Retarded intermolecular interactions involving diamagnetic molecules

✍ Scribed by A. Salam

Publisher: John Wiley and Sons
Year: 2000
Tongue: English
Weight: 154 KB
Volume: 78
Category: Article
ISSN: 0020-7608
DOI: 10.1002/(sici)1097-461x(2000)78:6<437::aid-qua4>3.0.co;2-7

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✦ Synopsis

Second-and third-order time-dependent perturbation theory within the multipolar framework of nonrelativistic quantum electrodynamics is used to calculate the retarded dispersion interaction between two diamagnetic molecules, a diamagnetic molecule and a magnetic-dipole susceptible molecule, and a diamagnetic molecule and an electric-quadrupole polarizable molecule. New expressions for the energy shift valid for all intermolecular separation distances, R, beyond the region of overlap of molecular electronic wave functions and applicable to a pair of randomly oriented molecules in the ground electronic state are given. The R-dependent behavior of the far-zone limit of the interaction energies is also examined.

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