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Relaxation of large molecules following ultrafast excitation

โœ Scribed by Andras Lorincz; Frank A. Novak; Stuart A. Rice

Publisher
Elsevier Science
Year
1984
Tongue
English
Weight
283 KB
Volume
111
Category
Article
ISSN
0009-2614

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โœฆ Synopsis

Wc deruonstrdte that the ulhfast rehation obxxvcd in the excited states oflargc org.mc molecules in solution m.~y bc understood 3s the collcrent evolution of the initlally prcparcd non-stationary state. It is shown that under fcmtosccond ewtt.tIion condtttons the relaxation is dctcrmincd by the chrxtcristics of the light pulse. The analysis of a simple pumpprobe cxlxrimcnt suggests rl way of me~surinp the chracteristics of ulrrxzhort pulses. The case of fluorescence cwited by ultrafJst puke\ is also dn.dyzcd.

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