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Reactivity of nucleophiles toward a p-benzyne derived from an enediyne

✍ Scribed by Charles L. Perrin; Gabriel J. Reyes-Rodríguez

Book ID
112175611
Publisher
John Wiley and Sons
Year
2012
Tongue
English
Weight
821 KB
Volume
26
Category
Article
ISSN
0894-3230

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Reactivity of a trivalent phosphorus rad
Reactivity of a trivalent phosphorus radical cation as an electrophile toward pyridine derivatives
✍ Shinro Yasui; Kosei Shioji; Munekazu Tsujimoto; Atsuyoshi Ohno 📂 Article 📅 2000 🏛 John Wiley and Sons 🌐 English ⚖ 185 KB

The reaction of methylviologen (MV ‫ם2‬ ) with tributylphosphine (1p) and diethylphenylphosphine (1q) in the presence of an alkyl-substituted pyridine (2) was found to take place through a singleelectron transfer (SET) from 1 to MV ‫ם2‬ followed by nucleophilic attack by 2 on the resulting phosphine