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Reactant rotational energy effect on energy distribution in products. The role of the electronic angular momentum

โœ Scribed by Y. Hurwitz; Y. Rudich; R. Naaman

Publisher
Elsevier Science
Year
1993
Tongue
English
Weight
618 KB
Volume
215
Category
Article
ISSN
0009-2614

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โœฆ Synopsis

In reactlons of 0( 'D) with CH4 clusters, CD4 and propane, monomers and clusters, preference for the 2II,,2 spm-orbit state of the OH product 1s observed New results on the effect of the mltlal rotational temperature of propane on the spin-orbit states dlstnbutlon are presented The preference for the *l-l ,I* state and the rotatlonal energy effect are attnbuted to conservation of electronic angular momentum during curve crossing m the entrance channel and to conservation of the projection of the electronic angular momentum on the Internuclear axis through the reaction A quantltatlve model ratlonahzes all the expenmental observations

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