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Quenching of UF6 (A state) by halomethanes

✍ Scribed by Fred B. Wampler; Richard C. Oldenborg; Walter W. Rice

Publisher: Elsevier Science
Year: 1979
Weight: 261 KB
Volume: 11
Category: Article
ISSN: 0047-2670
DOI: 10.1016/0047-2670(79)80058-1

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Rate constants at 25°C have been evaluated for the quenching of electronically excited UF 6 by selected organic molecules. Values for the rate constants at 25°C (units of 1011 R/mole s) for CH4, C2H6, C2F6, CHF2-CHF2, C2H2, and C2H4 are 0.061,3.8, 0.022, 0.072, 6.0, and 5, respectwely.

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UFs undergoes decomposition m the presence of SF6 when mixtures of both are madiated wrth a TEA CO2 laser. The mechanism for UFe decomposition may involve vrbrational energy transfer from excited SF, and laser absorption from the same laser pulse by excited UFe in its vibrational quasi-continuum \*

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