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Quantum interferences in the Ba⋯FCH3(B) + hν → BaF + CH3 intracluster reaction

✍ Scribed by K Gasmi; S Skowronek; A González Ureña

Publisher
Elsevier Science
Year
2003
Tongue
English
Weight
200 KB
Volume
376
Category
Article
ISSN
0009-2614

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✦ Synopsis

The laser-induced intracluster (BaÁ Á ÁFCH 3 ) + hm ! BaF à (Ba à ) + CH 3 (CH 3 F) bimolecular reaction has been investigated in the 17 780-18 750 cm À1 energy range, corresponding to the electronic B-state of the BaÁ Á ÁFCH 3 molecule. Both the photodepletion action spectrum and the action spectra of the reactive BaF and the non-reactive Ba photofragmentation channels were measured. The reaction probabilities of the two channels show an oscillatory behaviour with opposite phase. The oscillations in the energy dependence of both reactive and non-reactive probabilities for the cluster photofragmentation have been attributed to quantal interferences between the two photodissociation channels.

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